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Raft for mac free3/18/2023 With such a vast amount of literature, the RAFT process may appear a daunting topic to newcomers and nonexperts. To date, over 300 reviews have been published on RAFT polymerization, covering mechanistic understanding, polymer synthesis, and the numerous applications of materials obtained by RAFT. Today, with more than 8000 publications (see Figure 1 noticeably, the seminal paper on RAFT by the CSIRO group is to date the most cited article in Macromolecules, with over 3300 citations (5)), the RAFT process is a widely recognized polymerization technique, and it has been adopted by the wider scientific community, beyond polymer synthesis laboratories, as a tool to generate materials with a broad range of applications from materials science to medicine. The past 20 years have witnessed a rapidly growing interest in RAFT polymerization, initially focusing on the elucidation of the mechanism, then the demonstration of the myriad of polymeric architectures and functional materials that can be obtained from the process, and recently more application-driven reports. RDRP enables the synthesis of polymeric architectures exhibiting predictable molecular weight, low molar mass dispersity ( Đ), high end-group fidelity, and capacity for continued chain growth. RAFT is a reversible deactivation radical polymerization (RDRP), (4) also known as living or controlled radical polymerization-a process that mimics closely the feature of living polymerization while benefiting from the versatility of a radical process. Since its first report in 1998, (1-3) the reversible addition–fragmentation chain transfer (RAFT) process has grown into one of the most versatile and powerful polymerization techniques for the synthesis of complex polymeric architectures.
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